XUV Pump-Probe Experiments on Diatomic Molecules Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay /
This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is s...
| Published in: | Springer eBooks |
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| Format: | eBook |
| Language: | English |
| Published: |
Cham :
Springer International Publishing : Imprint: Springer,
2015.
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| Series: | Springer Theses, Recognizing Outstanding Ph.D. Research,
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| Subjects: | |
| Online Access: | http://dx.doi.org/10.1007/978-3-319-12139-0 Перейти в каталог НБ ТГУ |
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| 039 | 9 | |y 201702122144 |z Александр Эльверович Гилязов | |
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| 100 | 1 | |a Schnorr, Kirsten. |e author. |9 464002 | |
| 245 | 1 | 0 | |a XUV Pump-Probe Experiments on Diatomic Molecules |h electronic resource |b Tracing the Dynamics of Electron Rearrangement and Interatomic Coulombic Decay / |c by Kirsten Schnorr. |
| 260 | |a Cham : |b Springer International Publishing : |b Imprint: Springer, |c 2015. |9 742221 | ||
| 300 | |a XI, 191 p. 95 illus., 25 illus. in color. |b online resource. | ||
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| 490 | 1 | |a Springer Theses, Recognizing Outstanding Ph.D. Research, |x 2190-5053 | |
| 505 | 0 | |a Introduction -- Photoionization and Interatomic Coulombic Decay -- Free-Electron Lasers -- Experimental Setup -- Data Analysis -- Ionization Dynamics of I2 in XUV and IR Laser Pulses -- ICD Lifetime in Ne2 -- Conclusions and Outlook -- Appendices. | |
| 520 | |a This book explores the relaxation dynamics of inner-valence-ionized diatomic molecules on the basis of extreme-ultraviolet pump-probe experiments performed at the free-electron laser (FEL) in Hamburg. Firstly, the electron rearrangement dynamics in dissociating multiply charged iodine molecules is studied in an experiment that made it possible to access charge transfer in a thus far unexplored quasimolecular regime relevant for plasma and chemistry applications of the FEL. Secondly the lifetime of an efficient non-radiative relaxation process that occurs in weakly bound systems is measured directly for the first time in a neon dimer (Ne2). Interatomic Coulombic decay (ICD) has been identified as the dominant decay mechanism in inner-valence-ionized or excited van-der-Waals and hydrogen bonded systems, the latter being ubiquitous in all biomolecules. The role of ICD in DNA damage thus demands further investigation, e.g. with regard to applications like radiation therapy. | ||
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